In order to get the best out a fight, knowing a Type's weakness (see Lolimon Types) can help deal stronger hits, and so quick the process of weakening the Lolimon.
By choosing one of the already captured Lolimon, a fight can take place, which will weaken the Lolimon and make them more likely to be captured. If the latter is the chase, it shows a stronger type of ball is required, however if the former is true, the same type of ball could still have a chance. For example, a Lolimon could dodge it, or be too strong for it an bat it aside. Whilst Pokéballs (any type) are used to catch Lolimon, it is never really definite that the ball will hit the Lolimon in order to catch them. Despite this, Professor Eirin is still not sure that it will have 100% catch rate, and so labels it as "five times more likely to catch a Lolimon than a Pokéball" as an estimate. It was made from technology imported from the Lunar Capital, and is shown to successfully catch even the strongest of Lolimon. Whilst the Lunarian Ball is identical in appearance to the "Moon Ball" from Pokémon, it is actually very different. This can be used on much tougher foes, those recognised as being very strong Yōkai who even Reimu and Marisa can struggle to fight! However, it is shown that the strongest of the strong are more than a match for the Master Ball, leading to the eventual production of the "Lunarian Ball". Unlike in Pokémon, the Master Ball does not give a 100% chance to catching the target, but instead said to have "triple the chance of a Pokéball at catching a Lolimon". Whilst, like the Great Ball, these start off rare, more soon come as their production is mastered, and this allows Eirin to focus on creating an even better type of ball: the "Master Ball". These can be used on even tougher Lolimon, who are about average strength in the Touhou series, such as Reimu's allies (Aya, Reisen, Youmu, etc). The Ultra Ball is a superior version of the Great Ball, with a Lolimon "two times less likely to escape". Whilst at first Great Balls are far from abundant, with only three available, they are later placed on mass-production upon the creation of the "Ultra Ball".
Professor Eirin has created a new, stronger type of Pokéball called the "Great Ball" (basically the same as what is seen in Pokémon), making the Lolimon "1.5x less likely to escape". Fighting them will weaken them and make them easier to catch, however for even stronger Lolimon, stronger types of balls are required. However, upon meeting Professor Eirin, she explains that there are much tougher Lolimon who will require more than just a Pokéball to catch. Since the Lolimon first encountered are pretty weak, it seems they will do the job of collecting all the Lolimon. From the get go, there are an seemingly infinite amount of Pokéballs, that is, they don't seem to run out.
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